Using of supplement based on synthesized calcium hydrosilicates as structuring supplement in dry mixes lime is proposed. It shows the impact of supplement synthesis mode on the structure formation of calcareous compositions. X-ray analysis of lime samples based on synthesized supplements are presented. It is found that the mineralogical composition of the samples with the supplement of calcium hydrosilicates synthesized in the presence of diatomite is characterized by numerous peaks of low basic hydrosilicates and an increase in their intensity. The injection of supplements of hydrosilicates accelerates the gain of mechanical strength is established

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